Coherent rovibrational revivals in a thermal molecular ensemble. Bitter, M., Shapiro, E. A., & Milner, V. Physical Review A, 85(4):043410, American Physical Society, April, 2012. ![Coherent rovibrational revivals in a thermal molecular ensemble [link]](https://bibbase.org/img/filetypes/link.svg "link")
Paper doi abstract bibtex We report an experimental and theoretical study of the evolution of vibrational coherence in a thermal ensemble of nitrogen molecules. Rotational dephasing and rephasing of the vibrational coherence is detected by coherent anti-Stokes Raman scattering. The existence of rovibrational coupling and the discrete energy spectrum of the rotational bath lead to a whole new class of full and fractional rovibrational revivals. Following the rich rovibrational dynamics on a nanosecond time scale with subpicosecond time resolution enables us to determine the second-order rovibrational constant ?e and assess new possibilities of controlling decoherence.
@Article{Bitter2012a,
author = {Bitter, Martin and Shapiro, Evengy A. and Milner, Valery},
journal = {Physical Review A},
title = {Coherent rovibrational revivals in a thermal molecular ensemble},
year = {2012},
month = apr,
number = {4},
pages = {043410},
volume = {85},
abstract = {We report an experimental and theoretical study of the evolution of vibrational coherence in a thermal ensemble of nitrogen molecules. Rotational dephasing and rephasing of the vibrational coherence is detected by coherent anti-Stokes Raman scattering. The existence of rovibrational coupling and the discrete energy spectrum of the rotational bath lead to a whole new class of full and fractional rovibrational revivals. Following the rich rovibrational dynamics on a nanosecond time scale with subpicosecond time resolution enables us to determine the second-order rovibrational constant ?e and assess new possibilities of controlling decoherence.},
doi = {10.1103/PhysRevA.85.043410},
file = {Full Text PDF:https\://journals.aps.org/pra/pdf/10.1103/PhysRevA.85.043410:application/pdf;APS Snapshot:https\://journals.aps.org/pra/abstract/10.1103/PhysRevA.85.043410:text/html},
publisher = {American Physical Society},
url = {https://link.aps.org/doi/10.1103/PhysRevA.85.043410},
urldate = {2020-06-19TZ},
}
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