Amplification of impulsively excited molecular rotational coherence. Bustard, P., Sussman, B. b, & Walmsley, I. Physical Review Letters, 2010. Paper doi abstract bibtex We propose a scheme for preparation of high-coherence molecular dynamics which are phase stable with respect to ultrashort pulses. We experimentally demonstrate an example of this scheme using a phase-independent, nanosecond-duration, pump pulse to prepare a rotational coherence in molecular hydrogen. This rotational coherence is made phase stable with respect to a separate source of ultrashort pulses by seeding. The coherence is used to generate spectral broadening of femtosecond probe radiation by molecular phase modulation. © 2010 The American Physical Society.
@Article{Bustard2010,
author = {Bustard, P.J.a , Sussman, B.J.a b , Walmsley, I.A.a},
journal = {Physical Review Letters},
title = {Amplification of impulsively excited molecular rotational coherence},
year = {2010},
number = {19},
volume = {104},
abstract = {We propose a scheme for preparation of high-coherence molecular dynamics which are phase stable with respect to ultrashort pulses. We experimentally demonstrate an example of this scheme using a phase-independent, nanosecond-duration, pump pulse to prepare a rotational coherence in molecular hydrogen. This rotational coherence is made phase stable with respect to a separate source of ultrashort pulses by seeding. The coherence is used to generate spectral broadening of femtosecond probe radiation by molecular phase modulation. © 2010 The American Physical Society.},
affiliation = {Clarendon Laboratory, University of Oxford, Parks Road, Oxford, OX1 3PU, United Kingdom; Steacie Institute for Molecular Sciences, National Research Council of Canada, 100 Sussex Drive, Ottawa, ON K1A 0R6, Canada},
art_number = {193902},
document_type = {Article},
doi = {10.1103/PhysRevLett.104.193902},
source = {Scopus},
timestamp = {2016.03.02},
url = {http://www.scopus.com/inward/record.url?eid=2-s2.0-77952348703&partnerID=40&md5=cf38c215b512e2d300a97dfa7a5519ca},
}
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