Attosecond transient absorption spooktroscopy: a ghost imaging approach to ultrafast absorption spectroscopy. Driver, T., Li, S., Champenois, E. G, Duris, J., Ratner, D., Lane, T. J, Rosenberger, P., Al-Haddad, A., Averbukh, V., Barnard, T., Berrah, N., Bostedt, C., Bucksbaum, P. H, Coffee, R., Dimauro, L. F, Fang, L., Garratt, D., Gatton, A., Guo, Z., Hartmann, G., Haxton, D., Helml, W., Huang, Z., Laforge, A., Kamalov, A., Kling, M. F, Knurr, J., Lin, M., Lutman, A. A, Macarthur, J. P, Marangos, J. P, Nantel, M., Natan, A., Obaid, R., O'neal, J. T, Shivaram, N. H, Schori, A., Walter, P., Wang, A. L., Wolf, T. J A, Marinelli, A., & Cryan, J. P 2019. tex.ids: driver2020AttosecondTransientAbsorption publisher: The Royal Society of Chemistrydoi abstract bibtex The recent demonstration of isolated attosecond pulses from an X-ray free-electron laser (XFEL) opens the possibility for probing ultrafast electron dynamics at X-ray wavelengths. An established experimental method for probing ultrafast dynamics is X-ray transient absorption spectroscopy, where the X-ray absorption spectrum is measured by scanning the central photon energy and recording the resultant photoproducts. The spectral bandwidth inherent to attosecond pulses is wide compared to the resonant features typically probed, which generally precludes the application of this technique in the attosecond regime. In this paper we propose and demonstrate a new technique to conduct transient absorption spectroscopy with broad bandwidth attosecond pulses with the aid of ghost imaging, recovering sub-bandwidth resolution in photoproduct-based absorption measurements.
@article{driver_attosecond_2019,
title = {Attosecond transient absorption spooktroscopy: a ghost imaging approach to ultrafast absorption spectroscopy},
doi = {10.1039/c9cp03951a},
abstract = {The recent demonstration of isolated attosecond pulses from an X-ray free-electron laser (XFEL) opens the possibility for probing ultrafast electron dynamics at X-ray wavelengths. An established experimental method for probing ultrafast dynamics is X-ray transient absorption spectroscopy, where the X-ray absorption spectrum is measured by scanning the central photon energy and recording the resultant photoproducts. The spectral bandwidth inherent to attosecond pulses is wide compared to the resonant features typically probed, which generally precludes the application of this technique in the attosecond regime. In this paper we propose and demonstrate a new technique to conduct transient absorption spectroscopy with broad bandwidth attosecond pulses with the aid of ghost imaging, recovering sub-bandwidth resolution in photoproduct-based absorption measurements.},
urldate = {2020-01-27},
author = {Driver, Taran and Li, Siqi and Champenois, Elio G and Duris, Joseph and Ratner, Daniel and Lane, Thomas J and Rosenberger, Philipp and Al-Haddad, Andre and Averbukh, Vitali and Barnard, Toby and Berrah, Nora and Bostedt, Christoph and Bucksbaum, Philip H and Coffee, Ryan and Dimauro, Louis F and Fang, Li and Garratt, Douglas and Gatton, Averell and Guo, Zhaoheng and Hartmann, Gregor and Haxton, Daniel and Helml, Wolfram and Huang, Zhirong and Laforge, Aaron and Kamalov, Andrei and Kling, Matthias F and Knurr, Jonas and Lin, Ming-Fu and Lutman, Alberto A and Macarthur, James P and Marangos, Jon P and Nantel, Megan and Natan, Adi and Obaid, Razib and O'neal, Jordan T and Shivaram, Niranjan H and Schori, Aviad and Walter, Peter and Wang, Anna Li and Wolf, Thomas J A and Marinelli, Agostino and Cryan, James P},
year = {2019},
note = {tex.ids: driver2020AttosecondTransientAbsorption
publisher: The Royal Society of Chemistry},
}
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