Carbon Nanotube Nanoelectromechanical Systems as Magnetometers for Single-Molecule Magnets. Ganzhorn, M., Klyatskaya, S., Ruben, M., & Wernsdorfer, W. ACS Nano, 7(7):6225–6236, 2013.
Paper doi abstract bibtex Due to outstanding mechanical and electronic properties, carbon nanotube nanoelectromechanical systems (NEMS) were recently proposed as ultrasensitive magnetometers for single-molecule magnets (SMM). In this article, we describe a noninvasive grafting of a SMM on a carbon nanotube NEMS, which conserves both the mechanical properties of the carbon nanotube NEMS and the magnetic properties of the SMM. We will demonstrate that the nonlinearity of a carbon nanotube’s mechanical motion can be used to probe the reversal of a molecular spin, associated with a bis(phthalocyaninato)terbium(III) single-molecule magnet, providing an experimental evidence for the detection of a single spin by a mechanical degree of freedom on a molecular level.
@article{ganzhorn_carbon_2013,
title = {Carbon {Nanotube} {Nanoelectromechanical} {Systems} as {Magnetometers} for {Single}-{Molecule} {Magnets}},
volume = {7},
issn = {1936-0851},
url = {http://dx.doi.org/10.1021/nn402968k},
doi = {10.1021/nn402968k},
abstract = {Due to outstanding mechanical and electronic properties, carbon nanotube nanoelectromechanical systems (NEMS) were recently proposed as ultrasensitive magnetometers for single-molecule magnets (SMM). In this article, we describe a noninvasive grafting of a SMM on a carbon nanotube NEMS, which conserves both the mechanical properties of the carbon nanotube NEMS and the magnetic properties of the SMM. We will demonstrate that the nonlinearity of a carbon nanotube’s mechanical motion can be used to probe the reversal of a molecular spin, associated with a bis(phthalocyaninato)terbium(III) single-molecule magnet, providing an experimental evidence for the detection of a single spin by a mechanical degree of freedom on a molecular level.},
number = {7},
urldate = {2016-12-08},
journal = {ACS Nano},
author = {Ganzhorn, Marc and Klyatskaya, Svetlana and Ruben, Mario and Wernsdorfer, Wolfgang},
year = {2013},
pages = {6225--6236},
}
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