Organic Aerosol Yields from alpha-Pinene Oxidation: Bridging the Gap between First-Generation Yields and Aging Chemistry. Henry, K., M., Lohaus, T., & Donahue, N., M. Environmental Science & Technology, 46:12347-12354, 2012. ![Organic Aerosol Yields from alpha-Pinene Oxidation: Bridging the Gap between First-Generation Yields and Aging Chemistry [link]](https://bibbase.org/img/filetypes/link.svg "link")
Website abstract bibtex Secondary organic aerosol formation from volatile precursors can be thought of as a succession of generations of reaction products. Here, we constrain first-generation SOA formation from the alpha-pinene + OH reaction and also study SOA formation from alpha-pinene ozonolysis carried out without an OH scavenger. SOA yields from OH oxidation of alpha-pinene are significantly higher than SOA yields from ozonolysis including an OH scavenger, and the SOA mass yields for unscavenged ozonolysis generally fall within the range of mass yields for alpha-pinene ozonolysis under various conditions. Taken together, first-generation product yields parametrized with a volatility basis set fit provide a starting point for atmospheric models designed to simulate both the production and subsequent aging of SOA from this important terpene.
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abstract = {Secondary organic aerosol formation from volatile precursors can be thought of as a succession of generations of reaction products. Here, we constrain first-generation SOA formation from the alpha-pinene + OH reaction and also study SOA formation from alpha-pinene ozonolysis carried out without an OH scavenger. SOA yields from OH oxidation of alpha-pinene are significantly higher than SOA yields from ozonolysis including an OH scavenger, and the SOA mass yields for unscavenged ozonolysis generally fall within the range of mass yields for alpha-pinene ozonolysis under various conditions. Taken together, first-generation product yields parametrized with a volatility basis set fit provide a starting point for atmospheric models designed to simulate both the production and subsequent aging of SOA from this important terpene.},
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author = {Henry, K M and Lohaus, T and Donahue, N M},
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