Evaluation of nucleation theories in a sulfur-rich environment

Evaluation of nucleation theories in a sulfur-rich environment. Jung, Gun, J., Pandis, S. N., & Adams, P. J. Aerosol Science and Technology, 42(7):495-504, TAYLOR \& FRANCIS INC, 325 CHESTNUT ST, SUITE 800, PHILADELPHIA, PA 19106 USA, 2008.
doi abstract bibtex

Six nucleation parameterizations are tested using the Dynamic Model for Aerosol Nucleation (DMAN). Weak, moderate, and strong nucleation events together with days without nucleation from the Pittsburgh Air Quality Study (PAQS) were selected for the evaluation. The ability of the different theories to reproduce the occurrence or lack of a nucleation event was evaluated. The ternary sulfuric acid-ammonia-water theory was the only one that was successful for all tests. Sensitivity tests of the remaining parameterizations suggest that increasing or decreasing the corresponding nucleation rates does not change the overall performance of the parameterizations when both the nucleation and non-nucleation days are included in the tests.

@article{ Jung:ast:2008a,
  abstract = {Six nucleation parameterizations are tested using the Dynamic Model for Aerosol Nucleation (DMAN). Weak, moderate, and strong nucleation events together with days without nucleation from the Pittsburgh Air Quality Study (PAQS) were selected for the evaluation. The ability of the different theories to reproduce the occurrence or lack of a nucleation event was evaluated. The ternary sulfuric acid-ammonia-water theory was the only one that was successful for all tests. Sensitivity tests of the remaining parameterizations suggest that increasing or decreasing the corresponding nucleation rates does not change the overall performance of the parameterizations when both the nucleation and non-nucleation days are included in the tests.},
  address = {325 CHESTNUT ST, SUITE 800, PHILADELPHIA, PA 19106 USA},
  author = {Jung, Jae Gun and Pandis, Spyros N. and Adams, Peter J.},
  date = {2008},
  date-added = {2008-11-26 13:58:23 +0100},
  date-modified = {2008-11-26 14:02:04 +0100},
  doi = {DOI 10.1080/02786820802187085},
  isi = {000257152500001},
  isi-recid = {171785321},
  isi-ref-recids = {128079439 129111781 70145969 108704368 128074550 112242469 108917606 136448151 108543207 91107924 105563435 125778958 149195580 99612440 142822841 87318086 119876121 97400069 95802784 72789614 121638259 149693198 157429256 114723036 171511024 171511025 112722107 149145079 128079389 114007675 104882490 133750306 136448150 128173179 111114355 134405963 150536339 92553947 99840718 171511026 128079483 122778974 122778972 121638266 81966222 155884270 89077305 171511027 153674836 134927045 134834582 171511028 49348657 104208766 25972025 128276569 108722054 106154802 134926968 119028113 153249429 152877276 128276875 134715980},
  journal = {Aerosol Science and Technology},
  number = {7},
  pages = {495-504},
  publisher = {TAYLOR \& FRANCIS INC},
  timescited = {0},
  title = {Evaluation of nucleation theories in a sulfur-rich environment},
  volume = {42},
  year = {2008},
  bdsk-url-1 = {http://gateway.isiknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcAuth=Alerting&SrcApp=Alerting&DestApp=WOS&DestLinkType=FullRecord;KeyUT=000257152500001}
}

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