The time evolution of aerosol size distribution over the Mexico City plateau. Kleinman, L., I., Springston, S., R., Wang, J., Daum, P., H., Lee, Y., N., Nunnermacker, L., J., Senum, G., I., Weinstein-Lloyd, J., Alexander, M., L., Hubbe, J., Ortega, J., Zaveri, R., a., Canagaratna, M., R., & Jayne, J. Atmospheric Chemistry and Physics, 9(13):4261-4278, 2009.
Paper
Website abstract bibtex As part of the MILAGRO field campaign, the DOE G-1 aircraft was used to make measurements over and downwind of Mexico City with the objective of determining growth characteristics of aerosols from a megacity urban source. This study focuses on number concentration and size distributions. It is found that a 5-fold increase in aerosol volume is accompanied by about a 5-fold increase in accumulation mode number concentration. There is growth in aerosol volume because there are more accumulation mode particles, not because of an increase in the average size of accumulation particles. Condensation and volume growth laws were examined to see whether either is consistent with observations. Condensation calculations show that the growth of Aitken mode particles into the accumulation mode size range gives the required increase in number concentration. There are minimal changes in the accumulation mode size distribution with age, consistent with observations. Volume-growth in contrast yields a population of large particles, distinctly different from what is observed. Detailed model calculations are required to translate our observations into specific information on the volatility and properties of secondary organic aerosol.
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title = {The time evolution of aerosol size distribution over the Mexico City plateau},
type = {article},
year = {2009},
identifiers = {[object Object]},
keywords = {aerodynamic diameter measurements,atmosphere,campaign,chemistry,climate,combined mobility,density characterization,emissions,growth,mass-spectrometer,mechanisms,metropolitan-area,model,particle morphology,secondary organic aerosol,volatility},
pages = {4261-4278},
volume = {9},
websites = {<Go to ISI>://000267984400005,<Go to ISI>://000254416700007},
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notes = {<b>From Duplicate 1 (<i>The time evolution of aerosol size distribution over the Mexico City plateau</i> - Kleinman, L I; Springston, S R; Wang, J; Daum, P H; Lee, Y N; Nunnermacker, L J; Senum, G I; Weinstein-Lloyd, J; Alexander, M L; Hubbe, J; Ortega, J; Zaveri, R A; Canagaratna, M R; Jayne, J)<br/></b><br/>470OG<br/>Times Cited:8<br/>Cited References Count:48<br/><br/><b>From Duplicate 2 (<i>The time evolution of aerosol size distribution over the Mexico City plateau</i> - Kleinman, L. I.; Springston, S. R.; Wang, J.; Daum, P. H.; Lee, Y.-N.; Nunnermacker, L. J.; Senum, G. I.; Weinstein-Lloyd, J.; Alexander, M. L.; Hubbe, J.; Ortega, J.; Zaveri, R. a.; Canagaratna, M. R.; Jayne, J.)<br/></b><br/><b>From Duplicate 1 (<i>The time evolution of aerosol size distribution over the Mexico City plateau</i> - Kleinman, L. I.; Springston, S. R.; Wang, J.; Daum, P. H.; Lee, Y.-N.; Nunnermacker, L. J.; Senum, G. I.; Weinstein-Lloyd, J.; Alexander, M. L.; Hubbe, J.; Ortega, J.; Zaveri, R. a.; Canagaratna, M. R.; Jayne, J.)<br/></b><br/>280HN<br/>Times Cited:52<br/>Cited References Count:55<br/><br/><b>From Duplicate 2 (<i>The time evolution of aerosol size distribution over the Mexico City plateau</i> - Kleinman, L. I.; Springston, S. R.; Wang, J.; Daum, P. H.; Lee, Y.-N.; Nunnermacker, L. J.; Senum, G. I.; Weinstein-Lloyd, J.; Alexander, M. L.; Hubbe, J.; Ortega, J.; Zaveri, R. a.; Canagaratna, M. R.; Jayne, J.)<br/></b><br/>470OG<br/>Times Cited:8<br/>Cited References Count:48},
abstract = {As part of the MILAGRO field campaign, the DOE G-1 aircraft was used to make measurements over and downwind of Mexico City with the objective of determining growth characteristics of aerosols from a megacity urban source. This study focuses on number concentration and size distributions. It is found that a 5-fold increase in aerosol volume is accompanied by about a 5-fold increase in accumulation mode number concentration. There is growth in aerosol volume because there are more accumulation mode particles, not because of an increase in the average size of accumulation particles. Condensation and volume growth laws were examined to see whether either is consistent with observations. Condensation calculations show that the growth of Aitken mode particles into the accumulation mode size range gives the required increase in number concentration. There are minimal changes in the accumulation mode size distribution with age, consistent with observations. Volume-growth in contrast yields a population of large particles, distinctly different from what is observed. Detailed model calculations are required to translate our observations into specific information on the volatility and properties of secondary organic aerosol.},
bibtype = {article},
author = {Kleinman, L. I. and Springston, S. R. and Wang, J. and Daum, P. H. and Lee, Y.-N. N and Nunnermacker, L. J. and Senum, G. I. and Weinstein-Lloyd, J. and Alexander, M. L. and Hubbe, J. and Ortega, J. and Zaveri, R. a. and Canagaratna, M. R. and Jayne, J.},
journal = {Atmospheric Chemistry and Physics},
number = {13}
}
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