Direct observations of atmospheric aerosol nucleation. Kulmala, M., Kontkanen, J., Junninen, H., Lehtipalo, K., Manninen, H., E., Nieminen, T., Petäjä, T., Sipilä, M., Schobesberger, S., Rantala, P., Franchin, A., Jokinen, T., Järvinen, E., Äijälä, M., Kangasluoma, J., Hakala, J., Aalto, P., P., Paasonen, P., Mikkilä, J., Vanhanen, J., Aalto, J., Hakola, H., Makkonen, U., Ruuskanen, T., Mauldin, R., L., Duplissy, J., Vehkamäki, H., Bäck, J., Kortelainen, A., Riipinen, I., Kurtén, T., Johnston, M., V., Smith, J., N., Ehn, M., Mentel, T., F., Lehtinen, K., E., Laaksonen, A., Kerminen, V., M., & Worsnop, D., R. Science, 339(6122):943-946, 2013.
Direct observations of atmospheric aerosol nucleation [link]Website  doi  abstract   bibtex   
Atmospheric nucleation is the dominant source of aerosol particles in the global atmosphere and an important player in aerosol climatic effects. The key steps of this process occur in the sub-2-nanometer (nm) size range, in which direct size-segregated observations have not been possible until very recently. Here, we present detailed observations of atmospheric nanoparticles and clusters down to 1-nm mobility diameter. We identified three separate size regimes below 2-nm diameter that build up a physically, chemically, and dynamically consistent framework on atmospheric nucleation - more specifically, aerosol formation via neutral pathways. Our findings emphasize the important role of organic compounds in atmospheric aerosol formation, subsequent aerosol growth, radiative forcing and associated feedbacks between biogenic emissions, clouds, and climate.
@article{
 title = {Direct observations of atmospheric aerosol nucleation},
 type = {article},
 year = {2013},
 keywords = {amine,climate,clusters,growth,nanoparticles,particle formation,rates,smear-ii,sulfuric-acid,water},
 pages = {943-946},
 volume = {339},
 websites = {http://www.sciencemag.org/content/339/6122/943.abstract},
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 created = {2020-08-21T23:09:04.152Z},
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 last_modified = {2020-08-21T23:09:04.152Z},
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 citation_key = {Kulmala2013},
 source_type = {Journal Article},
 language = {English},
 notes = {<b>From Duplicate 1 (<i>Direct observations of atmospheric aerosol nucleation</i> - Kulmala, Markku; Kontkanen, Jenni; Junninen, Heikki; Lehtipalo, Katrianne; Manninen, Hanna E.; Nieminen, Tuomo; Petäjä, Tuukka; Sipilä, Mikko; Schobesberger, Siegfried; Rantala, Pekka; Franchin, Alessandro; Jokinen, Tuija; Järvinen, Emma; Äijälä, Mikko; Kangasluoma, Juha; Hakala, Jani; Aalto, Pasi P.; Paasonen, Pauli; Mikkilä, Jyri; Vanhanen, Joonas; Aalto, Juho; Hakola, Hannele; Makkonen, Ulla; Ruuskanen, Taina; Mauldin, Roy L.; Duplissy, Jonathan; Vehkamäki, Hanna; Bäck, Jaana; Kortelainen, Aki; Riipinen, Ilona; Kurtén, Theo; Johnston, Murray V.; Smith, James N.; Ehn, Mikael; Mentel, Thomas F.; Lehtinen, Kari E.J.; Laaksonen, Ari; Kerminen, Veli Matti; Worsnop, Douglas R.)<br/></b><br/>Times Cited: 123<br/><br/><b>From Duplicate 2 (<i>Direct observations of atmospheric aerosol nucleation</i> - Kulmala, Markku; Kontkanen, Jenni; Junninen, Heikki; Lehtipalo, Katrianne; Manninen, Hanna E.; Nieminen, Tuomo; Petäjä, Tuukka; Sipilä, Mikko; Schobesberger, Siegfried; Rantala, Pekka; Franchin, Alessandro; Jokinen, Tuija; Järvinen, Emma; Äijälä, Mikko; Kangasluoma, Juha; Hakala, Jani; Aalto, Pasi P.; Paasonen, Pauli; Mikkilä, Jyri; Vanhanen, Joonas; Aalto, Juho; Hakola, Hannele; Makkonen, Ulla; Ruuskanen, Taina; Mauldin, Roy L.; Duplissy, Jonathan; Vehkamäki, Hanna; Bäck, Jaana; Kortelainen, Aki; Riipinen, Ilona; Kurtén, Theo; Johnston, Murray V.; Smith, James N.; Ehn, Mikael; Mentel, Thomas F.; Lehtinen, Kari E.J.; Laaksonen, Ari; Kerminen, Veli Matti; Worsnop, Douglas R.)<br/></b><br/><b>From Duplicate 2 (<i>Direct Observations of Atmospheric Aerosol Nucleation</i> - Kulmala, M; Kontkanen, J; Junninen, H; Lehtipalo, K; Manninen, H E; Nieminen, T; Petaja, T; Sipila, M; Schobesberger, S; Rantala, P; Franchin, A; Jokinen, T; Jarvinen, E; Aijala, M; Kangasluoma, J; Hakala, J; Aalto, P P; Paasonen, P; Mikkila, J; Vanhanen, J; Aalto, J; Hakola, H; Makkonen, U; Ruuskanen, T; Mauldin, R L; Duplissy, J; Vehkamaki, H; Back, J; Kortelainen, A; Riipinen, I; Kurten, T; Johnston, M V; Smith, J N; Ehn, M; Mentel, T F; Lehtinen, K E J; Laaksonen, A; Kerminen, V M; Worsnop, D R)<br/></b><br/>Times Cited: 41<br/>Kulmala, Markku Kontkanen, Jenni Junninen, Heikki Lehtipalo, Katrianne Manninen, Hanna E. Nieminen, Tuomo Petaja, Tuukka Sipila, Mikko Schobesberger, Siegfried Rantala, Pekka Franchin, Alessandro Jokinen, Tuija Jarvinen, Emma Aijala, Mikko Kangasluoma, Juha Hakala, Jani Aalto, Pasi P. Paasonen, Pauli Mikkila, Jyri Vanhanen, Joonas Aalto, Juho Hakola, Hannele Makkonen, Ulla Ruuskanen, Taina Mauldin, Roy L., III Duplissy, Jonathan Vehkamaki, Hanna Back, Jaana Kortelainen, Aki Riipinen, Ilona Kurten, Theo Johnston, Murray V. Smith, James N. Ehn, Mikael Mentel, Thomas F. Lehtinen, Kari E. J. Laaksonen, Ari Kerminen, Veli-Matti Worsnop, Douglas R.<br/><br/><b>From Duplicate 3 (<i>Direct Observations of Atmospheric Aerosol Nucleation</i> - Kulmala, M; Kontkanen, J; Junninen, H; Lehtipalo, K; Manninen, H E; Nieminen, T; Petaja, T; Sipila, M; Schobesberger, S; Rantala, P; Franchin, A; Jokinen, T; Jarvinen, E; Aijala, M; Kangasluoma, J; Hakala, J; Aalto, P P; Paasonen, P; Mikkila, J; Vanhanen, J; Aalto, J; Hakola, H; Makkonen, U; Ruuskanen, T; Mauldin, R L; Duplissy, J; Vehkamaki, H; Back, J; Kortelainen, A; Riipinen, I; Kurten, T; Johnston, M V; Smith, J N; Ehn, M; Mentel, T F; Lehtinen, K E J; Laaksonen, A; Kerminen, V M; Worsnop, D R)<br/></b><br/>092UX<br/>Times Cited:1<br/>Cited References Count:31<br/><br/><b>From Duplicate 4 (<i>Direct observations of atmospheric aerosol nucleation</i> - Kulmala, Markku; Kontkanen, Jenni; Junninen, Heikki; Lehtipalo, Katrianne; Manninen, Hanna E.; Nieminen, Tuomo; Petäjä, Tuukka; Sipilä, Mikko; Schobesberger, Siegfried; Rantala, Pekka; Franchin, Alessandro; Jokinen, Tuija; Järvinen, Emma; Äijälä, Mikko; Kangasluoma, Juha; Hakala, Jani; Aalto, Pasi P.; Paasonen, Pauli; Mikkilä, Jyri; Vanhanen, Joonas; Aalto, Juho; Hakola, Hannele; Makkonen, Ulla; Ruuskanen, Taina; Mauldin, Roy L.; Duplissy, Jonathan; Vehkamäki, Hanna; Bäck, Jaana; Kortelainen, Aki; Riipinen, Ilona; Kurtén, Theo; Johnston, Murray V.; Smith, James N.; Ehn, Mikael; Mentel, Thomas F.; Lehtinen, Kari E.J.; Laaksonen, Ari; Kerminen, Veli Matti; Worsnop, Douglas R.)<br/></b><br/>Times Cited: 123},
 private_publication = {false},
 abstract = {Atmospheric nucleation is the dominant source of aerosol particles in the global atmosphere and an important player in aerosol climatic effects. The key steps of this process occur in the sub-2-nanometer (nm) size range, in which direct size-segregated observations have not been possible until very recently. Here, we present detailed observations of atmospheric nanoparticles and clusters down to 1-nm mobility diameter. We identified three separate size regimes below 2-nm diameter that build up a physically, chemically, and dynamically consistent framework on atmospheric nucleation - more specifically, aerosol formation via neutral pathways. Our findings emphasize the important role of organic compounds in atmospheric aerosol formation, subsequent aerosol growth, radiative forcing and associated feedbacks between biogenic emissions, clouds, and climate.},
 bibtype = {article},
 author = {Kulmala, Markku and Kontkanen, Jenni and Junninen, Heikki and Lehtipalo, Katrianne and Manninen, Hanna E. and Nieminen, Tuomo and Petäjä, Tuukka and Sipilä, Mikko and Schobesberger, Siegfried and Rantala, Pekka and Franchin, Alessandro and Jokinen, Tuija and Järvinen, Emma and Äijälä, Mikko and Kangasluoma, Juha and Hakala, Jani and Aalto, Pasi P. and Paasonen, Pauli and Mikkilä, Jyri and Vanhanen, Joonas and Aalto, Juho and Hakola, Hannele and Makkonen, Ulla and Ruuskanen, Taina and Mauldin, Roy L. and Duplissy, Jonathan and Vehkamäki, Hanna and Bäck, Jaana and Kortelainen, Aki and Riipinen, Ilona and Kurtén, Theo and Johnston, Murray V. and Smith, James N. and Ehn, Mikael and Mentel, Thomas F. and Lehtinen, Kari E.J. and Laaksonen, Ari and Kerminen, Veli Matti and Worsnop, Douglas R.},
 doi = {10.1126/science.1227385},
 journal = {Science},
 number = {6122}
}

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