Traditional Semiconductors in the Two-Dimensional Limit. Lucking, M. C., Xie, W., Choe, D., West, D., Lu, T., & Zhang, S. Physical Review Letters, 120(8):086101, February, 2018. Paper doi abstract bibtex Interest in two-dimensional materials has exploded in recent years. Not only are they studied due to their novel electronic properties, such as the emergent Dirac fermion in graphene, but also as a new paradigm in which stacking layers of distinct two-dimensional materials may enable different functionality or devices. Here, through first-principles theory, we reveal a large new class of two-dimensional materials which are derived from traditional III-V, II-VI, and I-VII semiconductors. It is found that in the ultrathin limit the great majority of traditional binary semiconductors studied (a series of 28 semiconductors) are not only kinetically stable in a two-dimensional double layer honeycomb structure, but more energetically stable than the truncated wurtzite or zinc-blende structures associated with three dimensional bulk. These findings both greatly increase the landscape of two-dimensional materials and also demonstrate that in the double layer honeycomb form, even ordinary semiconductors, such as GaAs, can exhibit exotic topological properties.
@article{lucking_traditional_2018,
title = {Traditional {Semiconductors} in the {Two}-{Dimensional} {Limit}},
volume = {120},
url = {https://link.aps.org/doi/10.1103/PhysRevLett.120.086101},
doi = {10.1103/PhysRevLett.120.086101},
abstract = {Interest in two-dimensional materials has exploded in recent years. Not only are they studied due to their novel electronic properties, such as the emergent Dirac fermion in graphene, but also as a new paradigm in which stacking layers of distinct two-dimensional materials may enable different functionality or devices. Here, through first-principles theory, we reveal a large new class of two-dimensional materials which are derived from traditional III-V, II-VI, and I-VII semiconductors. It is found that in the ultrathin limit the great majority of traditional binary semiconductors studied (a series of 28 semiconductors) are not only kinetically stable in a two-dimensional double layer honeycomb structure, but more energetically stable than the truncated wurtzite or zinc-blende structures associated with three dimensional bulk. These findings both greatly increase the landscape of two-dimensional materials and also demonstrate that in the double layer honeycomb form, even ordinary semiconductors, such as GaAs, can exhibit exotic topological properties.},
number = {8},
urldate = {2020-06-28},
journal = {Physical Review Letters},
author = {Lucking, Michael C. and Xie, Weiyu and Choe, Duk-Hyun and West, Damien and Lu, Toh-Ming and Zhang, S. B.},
month = feb,
year = {2018},
pages = {086101},
}
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