Non-Thermal Plasma Activation of Gold-Based Catalysts for Low-Temperature Water–Gas Shift Catalysis. Stere, C., Anderson, J., Chansai, S., Delgado, J., Goguet, A., Graham, W., Hardacre, C., Taylor, S., Tu, X., Wang, Z., & Yang, H. Angewandte Chemie - International Edition, 56(20):5579-5583, 2017. cited By 35![Non-Thermal Plasma Activation of Gold-Based Catalysts for Low-Temperature Water–Gas Shift Catalysis [link]](https://bibbase.org/img/filetypes/link.svg "link")
Paper doi abstract bibtex Non-thermal plasma activation has been used to enable low-temperature water-gas shift over a Au/CeZrO4 catalyst. The activity obtained was comparable with that attained by heating the catalyst to 180 °C providing an opportunity for the hydrogen production to be obtained under conditions where the thermodynamic limitations are minimal. Using in situ diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS), structural changes associated with the gold nanoparticles in the catalyst have been observed which are not found under thermal activation indicating a weakening of the Au−CO bond and a change in the mechanism of deactivation. © 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim
@ARTICLE{Stere20175579,
author={Stere, C.E. and Anderson, J.A. and Chansai, S. and Delgado, J.J. and Goguet, A. and Graham, W.G. and Hardacre, C. and Taylor, S.F.R. and Tu, X. and Wang, Z. and Yang, H.},
title={Non-Thermal Plasma Activation of Gold-Based Catalysts for Low-Temperature Water–Gas Shift Catalysis},
journal={Angewandte Chemie - International Edition},
year={2017},
volume={56},
number={20},
pages={5579-5583},
doi={10.1002/anie.201612370},
note={cited By 35},
url={https://www.scopus.com/inward/record.uri?eid=2-s2.0-85017653350&doi=10.1002%2fanie.201612370&partnerID=40&md5=bcb6da805e2e900bf10ba7dfb5a59313},
abstract={Non-thermal plasma activation has been used to enable low-temperature water-gas shift over a Au/CeZrO4 catalyst. The activity obtained was comparable with that attained by heating the catalyst to 180 °C providing an opportunity for the hydrogen production to be obtained under conditions where the thermodynamic limitations are minimal. Using in situ diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS), structural changes associated with the gold nanoparticles in the catalyst have been observed which are not found under thermal activation indicating a weakening of the Au−CO bond and a change in the mechanism of deactivation. © 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim},
keywords={Carbon; Carbon monoxide; Catalysis; Catalyst activity; Catalysts; Chemical activation; Chemical shift; Fourier transform infrared spectroscopy; Gold; Hydrogen production; Temperature, Diffuse reflectance infrared fourier transform spectroscopies; Gold Nanoparticles; Low-temperature water-gas shift; Nonthermal plasma; Plasma catalysis; Thermal activation; Thermodynamic equilibria; Water gas shift (WGS) reaction, Water gas shift},
document_type={Article},
source={Scopus},
}
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